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I think in general, there are a couple things to look at when comparing molecules. The first is the state each molecule occupies, as we know that Sgas>Sliquid>Ssolid. Additionally, it is important to compare the relative size of the molecule, as an increase in the number of bonds and electrons leads to higher positional entropy. Also, deltaS increases with molar complexity, so looking at the atomic structures would also give you some direction.
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